I assume you're talking about those very rare one-of-a-kind songs (often, if not only, mellow instrumentals) which exist that are sonic gems and not necessarily personal favorites that appeal to one's subjective taste in music.
A truly spiritually uplifting and cocooning song that immediately comes to mind and which I find to be quite divinely atmospheric and transporting is from the excellent Dan Gibson Solitudes series:
Album: In The Midst Of Angels
Track: 2 ("Canyon Legacy")
The beautiful chorales are lovely and enchanting and in my opinion this is the type of sound that would most likely be heard in heaven.
I enjoy a variety of music, including (more uptempo) genres I like better than this, but to answer your question, I can only think of a few instrumentals that best capture the heavenly spirit, with this being one of them.
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